Visible light assisted heterogeneous electro-fenton oxidation of catechol catalyzed by nano-Fe3O4

Baolin Hou, Ye Liu, Bozhi Ren, Andrew S. Hursthouse

Research output: Contribution to journalArticle

Abstract

Degradation of catechol in visible light assisted heterogeneous electro-Fenton catalyzed by nano-Fe3O4 was study and the effects of operational parameters such as current density, temperature, illumination intensity and catalyst dosage on degradation performance were investigated respectively. The prepared nano-Fe3O4 catalyst was characterized with SEM, XRD et. al. Efficient degradation performance was obtained in this visible light assisted heterogeneous electro-Fenton system. The relationship between apparent rate constant and catalyst dosage at lower values exhibited high relativity. The interface reaction mechanism was dominant in this heterogeneous system catalyzed by nano-Fe3O4 based on the normalization of apparent rate constant and thermodynamics analysis. In addition, the stability and reusability of the prepared catalyst was tested via successive bath experiments.
Original languageEnglish
Pages (from-to)1681-1687
Number of pages7
JournalFresenius Environmental Bulletin
Volume27
Issue number3
Publication statusPublished - 1 Mar 2018

Fingerprint

Electrooxidation
catalyst
oxidation
Catalysts
Degradation
degradation
Rate constants
Relativity
Reusability
Current density
thermodynamics
Lighting
scanning electron microscopy
X-ray diffraction
Thermodynamics
Scanning electron microscopy
catechol
experiment
temperature
Experiments

Keywords

  • heterogeneous electro-Fenton
  • nano-Fe3O4
  • visible light assisted
  • catechol

Cite this

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abstract = "Degradation of catechol in visible light assisted heterogeneous electro-Fenton catalyzed by nano-Fe3O4 was study and the effects of operational parameters such as current density, temperature, illumination intensity and catalyst dosage on degradation performance were investigated respectively. The prepared nano-Fe3O4 catalyst was characterized with SEM, XRD et. al. Efficient degradation performance was obtained in this visible light assisted heterogeneous electro-Fenton system. The relationship between apparent rate constant and catalyst dosage at lower values exhibited high relativity. The interface reaction mechanism was dominant in this heterogeneous system catalyzed by nano-Fe3O4 based on the normalization of apparent rate constant and thermodynamics analysis. In addition, the stability and reusability of the prepared catalyst was tested via successive bath experiments.",
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Visible light assisted heterogeneous electro-fenton oxidation of catechol catalyzed by nano-Fe3O4. / Hou, Baolin; Liu, Ye; Ren, Bozhi; Hursthouse, Andrew S.

In: Fresenius Environmental Bulletin, Vol. 27, No. 3, 01.03.2018, p. 1681-1687.

Research output: Contribution to journalArticle

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T1 - Visible light assisted heterogeneous electro-fenton oxidation of catechol catalyzed by nano-Fe3O4

AU - Hou, Baolin

AU - Liu, Ye

AU - Ren, Bozhi

AU - Hursthouse, Andrew S.

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AB - Degradation of catechol in visible light assisted heterogeneous electro-Fenton catalyzed by nano-Fe3O4 was study and the effects of operational parameters such as current density, temperature, illumination intensity and catalyst dosage on degradation performance were investigated respectively. The prepared nano-Fe3O4 catalyst was characterized with SEM, XRD et. al. Efficient degradation performance was obtained in this visible light assisted heterogeneous electro-Fenton system. The relationship between apparent rate constant and catalyst dosage at lower values exhibited high relativity. The interface reaction mechanism was dominant in this heterogeneous system catalyzed by nano-Fe3O4 based on the normalization of apparent rate constant and thermodynamics analysis. In addition, the stability and reusability of the prepared catalyst was tested via successive bath experiments.

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